Non-Deterministic Phase Dynamics in Nanoparticles Enabled by Surface Energy

Non-Deterministic Phase Dynamics in Nanoparticles Enabled by Surface Energy



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English | April 18, 2026 | ISBN-10: 9819572177 | 80 pages| Epub PDF (True) | 43 MB

This thesis describes the development of in-situ cinematographic recording techniques for investigating phase dynamics using nanoparticles (NPs) as model systems. The suitable experimental platform realized the simultaneous high spatial and temporal resolution for in-situ observations of phase transitions. The impact of increased surface energy on phase stability in NPs drives phase dynamics under ambient conditions. By leveraging this, nano-specific polymorphs and the energy profile of structural fluctuation on NPs of inorganic compounds were identified at atomic resolution in real space. The surface energy-driven phase dynamics revealed here provide new guidelines for controlling nanomaterial structures and expanding the scope of future material exploration.

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